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Annual cycle of ozone at and above the tropical tropopause: observations versus simulations with the Chemical Lagrangian Model of the Stratosphere (CLaMS)

Item

Title (Dublin Core)

Annual cycle of ozone at and above the tropical tropopause: observations versus simulations with the Chemical Lagrangian Model of the Stratosphere (CLaMS)

Description (Dublin Core)

Multi-annual simulations with the Chemical Lagrangian Model of the Stratosphere (CLaMS) were conducted to study the seasonality of O<sub>3</sub> within the stratospheric part of the tropical tropopause layer (TTL), i.e. above &theta;=360 K potential temperature level. In agreement with satellite (HALOE) and in-situ observations (SHADOZ), CLaMS simulations show a pronounced annual cycle in O<sub>3</sub>, at and above &theta;=380 K, with the highest mixing ratios in the late boreal summer. Within the model, this cycle is driven by the seasonality of both upwelling and in-mixing. The latter process occurs through enhanced horizontal transport from the extratropics into the TTL that is mainly driven by the meridional, isentropic winds. The strongest in-mixing occurs during the late boreal summer from the Northern Hemisphere in the potential temperature range between 370 and 420 K. Complementary, the strongest upwelling occurs in winter reducing O<sub>3</sub> to the lowest values in early spring. Both CLaMS simulations and Aura MLS O<sub>3</sub> observations consistently show that enhanced in-mixing in summer is mainly driven by the Asian monsoon anticyclone.

Creator (Dublin Core)

Konopka, P.
Grooß, J.-U.
Günther, G.
Ploeger, F.
Pommrich, R.
Müller, R.
Livesey, N.

Date (Dublin Core)

2018-01-15

Type (Dublin Core)

Text

Format (Dublin Core)

application/pdf

Identifier (Dublin Core)

10.5194/acp-10-121-2010
https://acp.copernicus.org/articles/10/121/2010/

Source (Dublin Core)

eISSN: 1680-7324

Language (Dublin Core)

eng
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