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Strong spectral dependence of light absorption by organic carbon particles formed by propane combustion

Item

Title (Dublin Core)

Strong spectral dependence of light absorption by organic carbon particles formed by propane combustion

Description (Dublin Core)

We have measured the extinction and absorption cross sections of carbon particles emitted by a propane diffusion flame both in an aerosol chamber and on size-segregated samples deposited on optical windows. The absorption cross section, the single scattering albedo, and the Ångström exponent show drastic dependencies both on the C/O ratio and on the particle size. This is interpretated as being due to the appearance of nucleation modes of smaller organic particles at higher C/O ratios, which were detected by SMPS measurements and partially by TEM analysis. The spectral range of the validity of the absorption power-law (Ångström exponent) model is investigated by vacuum ultraviolet extinction measurements. These measurements give also indications for a preferentially aromatic nature of the OC component of the flame products.

Creator (Dublin Core)

Schnaiter, M.
Gimmler, M.
Llamas, I.
Linke, C.
Jäger, C.
Mutschke, H.

Date (Dublin Core)

2018-06-28

Type (Dublin Core)

Text

Format (Dublin Core)

application/pdf

Identifier (Dublin Core)

10.5194/acp-6-2981-2006
https://acp.copernicus.org/articles/6/2981/2006/

Source (Dublin Core)

eISSN: 1680-7324

Language (Dublin Core)

eng
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