Items

Advanced search

Lidar observations of middle atmosphere temperature variability

We discuss 223 middle atmosphere lidar temperature observations. The record was collected at Frascati (42°N–13°E), during the 41-month period January 1989-May 1992, corresponding to the maximum of solar cycle 22. The choice of this interval was aimed at minimizing the temperature variability induced by the 11-year solar cycle. The average climatology over the 41-month period and comparison with a reference atmosphere (CIRA86) are presented. Monthly temperature variability over the full period, during opposite quasi-biennial oscillation phases and on a short-term scale (0.5–4 h), is analyzed. Results indicate the 50–55-km region as less affected by variability caused by the natural phenomena considered in the analysis. Due to this minimum in natural noise characterizing the atmospheric temperature just above the stratopause, observations of that region are well suited to the detection of possible temperature trends induced by industrial activities.
Effect of Antarctic ozone holes of 1988, 1989, and 1990 on lower latitudes of the southern hemisphere

The October depletions in the Antarctic ozone spread to lower latitudes in early November in 1988, in late November in 1989, and in late October in 1990. The depletions were 10–15% for latitudes up to 40°S and smaller thereafter, and almost negligible at 25°S and beyond. However, for the southern hemisphere, the normal seasonal changes at middle latitudes from October to December are much larger (about 20%). Also, there are superposed fluctuations of about 20% over a few (5–6) days.
Interannual variability of United States cloudiness

United States cloudiness data for 1950–1992 show quasi-biennial (QBO) and quasi-triennial (QTO) oscillations which match partly with the QBO and QTO of the Southern Oscillation (SO) index (the Tahiti minus Darwin pressure), but not with the QBO of the 50-mb equatorial zonal wind. Cloudiness also shows significant periodicities near 4.2 and 7.5 years, and probably a sunspot cycle effect (periodicities 11–14 years), with minimum cloudiness at or soon after sunspot minima, though this could also be due to periodicities of 10 and 17 years observed in the SO index. During 1955–1970, cloudiness increased by about 1%. Thereafter, it remained almost steady for the eastern and central parts of the USA, but continued to rise until about 1980 for the western USA.
Variations in the strength of the Sq current system

The strength of the Sq current system is measured by taking the difference between magnetic variations on either side of the current system focus. This is carried out for several longitude sectors. A distinct semiannual variation is sometimes found but its incidence varies with longitude, local time and hemisphere. Other semiannual effects in the ionosphere are reviewed and the possibility of a diurnal modulation of the strength of the 12-h tide is suggested.
Diffusion spreading of middle-latitude ionospheric plasma irregularities

In contrast to the way that the spreading of irregularities in a plasma is usually considered, the diffusion spreading of irregularities stretched along the geomagnetic field B is examined using a three-dimensional rigorous numerical model of quasi-neutral diffusion in the presence of a magnetic field, in conjunction with the actual height variations of the diffusion and conductivity tensors in the ionosphere. A comparison with the earlier constructed approximate model of unipolar diffusion was made. As in the previous case, the same peculiarities of irregularity spreading in the inhomogeneous background ionospheric plasma were observed. The accuracy of the approximate model for describing the process of spreading of anisotropic ionospheric irregularities is established. Time relaxation effects of real heating-induced ionospheric irregularities on their scale transverse to B are presented using the approximate analytical model for the case of a quasi-homogeneous ionospheric plasma. The calculated results have a vivid physical meaning and can be directly compared with experimental data on the radiophysical observations of artificial heating-induced irregularities created by powerful radio waves in the ionosphere.
Cloud ice caused by atmospheric mineral dust – Part 1: Parameterization of ice nuclei concentration in the NMME-DREAM model

Dust aerosols are very efficient ice nuclei, important for heterogeneous cloud glaciation even in regions distant from desert sources. A new generation of ice nucleation parameterizations, including dust as an ice nucleation agent, opens the way towards a more accurate treatment of cold cloud formation in atmospheric models. Using such parameterizations, we have developed a regional dust-atmospheric modelling system capable of predicting, in real time, dust-induced ice nucleation. We executed the model with the added ice nucleation component over the Mediterranean region, exposed to moderate Saharan dust transport, over two periods lasting 15 and 9 days, respectively. The model results were compared against satellite and ground-based cloud-ice-related measurements, provided by SEVIRI (Spinning Enhanced Visible and InfraRed Imager) and the CNR-IMAA Atmospheric Observatory (CIAO) in Potenza, southern Italy. The predicted ice nuclei concentration showed a reasonable level of agreement when compared against the observed spatial and temporal patterns of cloud ice water. The developed methodology permits the use of ice nuclei as input into the cloud microphysics schemes of atmospheric models, assuming that this approach could improve the predictions of cloud formation and associated precipitation.
Precipitation susceptibility in marine stratocumulus and shallow cumulus from airborne measurements

Precipitation tends to decrease as aerosol concentration increases in warm marine boundary layer clouds at fixed liquid water path (LWP). The quantitative nature of this relationship is captured using the precipitation susceptibility (So) metric. Previously published works disagree on the qualitative behavior of So in marine low clouds: So decreases monotonically with increasing LWP or cloud depth (H) in stratocumulus clouds (Sc), while it increases and then decreases in shallow cumulus clouds (Cu). This study uses airborne measurements from four field campaigns on Cu and Sc with similar instrument packages and flight maneuvers to examine if and why So behavior varies as a function of cloud type. The findings show that So increases with H and then decreases in both Sc and Cu. Possible reasons for why these results differ from those in previous studies of Sc are discussed.
Impacts of the 2014–2015 Holuhraun eruption on the UK atmosphere

Volcanic emissions, specifically from Iceland, pose a pan-European risk and are on the UK National Risk Register due to potential impacts on aviation, public health, agriculture, the environment and the economy, from both effusive and explosive activity. During the 2014–2015 fissure eruption at Holuhraun in Iceland, the UK atmosphere was significantly perturbed. This study focuses one major incursion in September 2014, affecting the surface concentrations of both aerosols and gases across the UK, with sites in Scotland experiencing the highest sulfur dioxide (SO2) concentrations. The perturbation event observed was confirmed to originate from the fissure eruption using satellite data from GOME2B and the chemical transport model, EMEP4UK, which was used to establish the spatial distribution of the plume over the UK during the event of interest. At the two UK European Monitoring and Evaluation Program (EMEP) supersite observatories (Auchencorth Moss, SE Scotland, and Harwell, SE England) significant alterations in sulfate (SO42−) content of PM10 and PM2.5 during this event, concurrently with evidence of an increase in ultrafine aerosol most likely due to nucleation and growth of aerosol within the plume, were observed. At Auchencorth Moss, higher hydrochloric acid (HCl) concentrations during the September event (max = 1.21 µg m−3, cf. annual average 0.12 µg m−3 in 2013), were assessed to be due to acid displacement of chloride (Cl−) from sea salt (NaCl) to form HCl gas rather than due to primary emissions of HCl from Holuhraun. The gas and aerosol partitioning at Auchencorth Moss of inorganic species by thermodynamic modelling confirmed the observed partitioning of HCl. Using the data from the chemical thermodynamic model, ISORROPIA-II, there is evidence that the background aerosol, which is typically basic at this site, became acidic with an estimated pH of 3.8 during the peak of the event. Volcano plume episodes were periodically observed by the majority of the UK air quality monitoring networks during the first 4 months of the eruption (August–December 2014), at both hourly and monthly resolution. In the low-resolution networks, which provide monthly SO2 averages, concentrations were found to be significantly elevated at remote “clean” sites in NE Scotland and SW England, with record-high SO2 concentrations for some sites in September 2014. For sites which are regularly influenced by anthropogenic emissions, taking into account the underlying trends, the eruption led to statistically unremarkable SO2 concentrations (return probabilities  > 0.1, ∼ 10 months). However, for a few sites, SO2 concentrations were clearly much higher than has been previously observed (return probability < 0.005, > 3000 months). The Holuhraun Icelandic eruption has resulted in a unique study providing direct evidence of atmospheric chemistry perturbation of both gases and aerosols in the UK background atmosphere. The measurements can be used to both challenge and verify existing atmospheric chemistry of volcano plumes, especially those originating from effusive eruptions, which have been underexplored due to limited observations available in the literature. If all European data sets were collated this would allow improved model verification and risk assessments for future volcanic eruptions of this type.
A comparative study of K-rich and Na/Ca-rich feldspar ice-nucleating particles in a nanoliter droplet freezing assay

A recently designed droplet freezing assay was used to study the freezing of up to 1500 identical 0.2 nL water droplets containing suspensions of one Na/Ca-rich feldspar and three K-rich and one Na/Ca-rich feldspar particles. Three types of experiments have been conducted: cooling ramp, isothermal freezing at a constant temperature, and freeze–thaw cycles. The observed freezing behavior has been interpreted with the help of a model based on the classical nucleation theory (soccer ball model (SBM); Niedermeier et al., 2015). By applying the model to the different freezing experiments conducted with the same ice-nucleating material, the unique sets of model parameters for specific feldspar suspensions could be derived. The SBM was shown to adequately describe the observed cooling rate dependence, the ice-nucleating active sites (INAS) surface density ns(T) in a wide temperature range, and the shift of the freezing curves towards lower temperature with dilution. Moreover, the SBM was capable of reproducing the variation of INAS surface density ns(T) with concentration of ice-nucleating particles in the suspension droplets and correctly predicting the leveling-off of ns(T) at low temperature. The freeze–thaw experiments have clearly shown that the heterogeneous freezing induced even by very active ice-nucleating species still possesses a stochastic nature, with the degree of randomness increasing towards homogeneous nucleation. A population of the high-temperature INAS has been identified in one of the K-rich feldspar samples. The freezing of 0.8 wt % suspension droplets of this particular feldspar was observed already at −5 °C. These high-temperature active sites could be deactivated by treating the sample with hydrogen peroxide but survived heating up to 90 °C. Given a high mass concentration of these high-temperature active sites (2.9 × 108 g−1) and a very low value of contact angle (0.56 rad) the possibility of biological contamination of the sample was concluded to be unlikely but could not be completely ruled out. The freezing efficacy of all feldspar samples has been shown to reduce only slightly after suspension in water for over 5 months.
A global catalogue of large SO2 sources and emissions derived from the Ozone Monitoring Instrument

Sulfur dioxide (SO2) measurements from the Ozone Monitoring Instrument (OMI) satellite sensor processed with the new principal component analysis (PCA) algorithm were used to detect large point emission sources or clusters of sources. The total of 491 continuously emitting point sources releasing from about 30 kt yr−1 to more than 4000 kt yr−1 of SO2 per year have been identified and grouped by country and by primary source origin: volcanoes (76 sources); power plants (297); smelters (53); and sources related to the oil and gas industry (65). The sources were identified using different methods, including through OMI measurements themselves applied to a new emission detection algorithm, and their evolution during the 2005–2014 period was traced by estimating annual emissions from each source. For volcanic sources, the study focused on continuous degassing, and emissions from explosive eruptions were excluded. Emissions from degassing volcanic sources were measured, many for the first time, and collectively they account for about 30 % of total SO2 emissions estimated from OMI measurements, but that fraction has increased in recent years given that cumulative global emissions from power plants and smelters are declining while emissions from oil and gas industry remained nearly constant. Anthropogenic emissions from the USA declined by 80 % over the 2005–2014 period as did emissions from western and central Europe, whereas emissions from India nearly doubled, and emissions from other large SO2-emitting regions (South Africa, Russia, Mexico, and the Middle East) remained fairly constant. In total, OMI-based estimates account for about a half of total reported anthropogenic SO2 emissions; the remaining half is likely related to sources emitting less than 30 kt yr−1 and not detected by OMI.